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As a result of the intensive studies to overcome the problems associated with the process of preparing L-carnitine, the invention herein has been devised based on the fact that the following reactions can be carried out with (S)-3-activated hydroxybutyrolactone as a raw material under the specific conditions: a ring-opening reaction, epoxydation where the chiral center is inversely converted, and nucleophilic substitution of trimethylamine